The pandemic and overlapping global crises, including climate change, have increased attention to the importance of mental health and well-being as foundational for humans. Similarly, COVID-19 significantly exacerbated gaps in education, leaving children one to three years behind. Artificial intelligence (AI) has demonstrated potential to be transformative in addressing challenges in mental health and education and in supporting broader sustainability issues. However, there are well-founded concerns about AI regarding its potential to exacerbate inequity, further marginalizing underserved communities. To further explore these issues, the National Academies of Sciences, Engineering, and Medicine's Roundtable on Science and Technology for Sustainability, in collaboration with the Board on Health Care Services and Board on Science Education, convened a hybrid workshop, Artificial Intelligence in Education and Mental Health for a Sustainable Future on May 30, 2024. The workshop consisted of two parts: AI in mental health and well-being and AI in education. Participants reviewed AI tools, applications, and strategies in education and mental health and the implications for sustainable development. The workshop also discussed AI's potential to accelerate progress on the Sustainable Development Goals.