The psychological harmony education, oriented to the unity of Truth, Good, Beauty, and in pursuit of a healthy, balanced and harmonious development of individual psychological quality to improve the mental quality, is an important part in mental education. In order to better fulfill the psychological harmony education of the college students, as well as guarantee this achievement, it should persist in the principles of wholeness and systematism, fully displaying the roles of Mental Health Education Center, teaching system, management system and environmental system. Besides, it should also pay more attention to the family education, social system and self-education of them.